Record Details

Radiation re-solution of fission gas in non-oxide nuclear fuel

ScholarsArchive at Oregon State University

Field Value
Title Radiation re-solution of fission gas in non-oxide nuclear fuel
Names Matthews, Christopher (creator)
Schwen, Daniel (creator)
Klein, Andrew C. (creator)
Date Issued 2015-02 (iso8601)
Note To the best of our knowledge, one or more authors of this paper were federal employees when contributing to this work. This is an author's peer-reviewed final manuscript, as accepted by the publisher. The published article is copyrighted by Elsevier and can be found at: http://www.journals.elsevier.com/journal-of-nuclear-materials.
Abstract Renewed interest in fast nuclear reactors is creating a need for better understanding of fission gas bubble behavior in non-oxide fuels. Collisions between
fission fragments and their subsequent cascades can knock fission gas atoms out
of bubbles and back into the fuel lattice, resulting in a loss term for the bubble.
By assuming these collisions can be treated as binary collisions, we calculated a
re-solution parameter as a function of bubble radius. The calculations showed
that there is a sharp decrease as bubble size increases until about 100 nm when
the re-solution parameter stays nearly constant. The bubble size dependence
may explain the large bubble size distribution found in some uranium carbide
and nitride fuels. Furthermore, our model shows ion cascades created in the
fuel result in many more implanted fission gas atoms than collisions directly
with fission fragments. Utilization of our calculated re-solution parameter can
be used to find a re-solution rate for future bubble behavior simulations.
Genre Article
Identifier Matthews, C., Schwen, D., & Klein, A. C. (2015). Radiation re-solution of fission gas in non-oxide nuclear fuel. Journal of Nuclear Materials, 457, 273-278. doi:10.1016/j.jnucmat.2014.11.108

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