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Pore-scale observations of supercritical CO₂ drainage in Bentheimer sandstone by synchrotron x-ray imaging

ScholarsArchive at Oregon State University

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Title Pore-scale observations of supercritical CO₂ drainage in Bentheimer sandstone by synchrotron x-ray imaging
Names Herring, Anna L. (creator)
Andersson, Linnea (creator)
Newell, D. L. (creator)
Carey, J. W. (creator)
Wildenschild, Dorthe (creator)
Date Issued 2014-06 (iso8601)
Note To the best of our knowledge, one or more authors of this paper were federal employees when contributing to this work. This is the publisher’s final pdf. The published article is copyrighted by Elsevier and can be found at: http://www.journals.elsevier.com/international-journal-of-greenhouse-gas-control.
Abstract This work utilizes synchrotron-based x-ray computed microtomography (x-ray CMT) imaging to quantify
the volume and topology of supercritical carbon dioxide (scCO₂) on a pore-scale basis throughout the
primary drainage process of a 6 mm diameter Bentheimer sandstone core. Experiments were performed
with brine and scCO₂ at 8.3 MPa (1200 psi) and 37.5°C. Capillary pressure–saturation curves for the scCO₂-brine system are presented and compared to the ambient air-brine system, and are shown to overlay one
another when pressure is normalized by interfacial tension. Results are analyzed from images with a
voxel resolution of 4.65 μm; image-based evidence demonstrates that scCO₂ invades the pore space in
a capillary fingering regime at a mobility ratio M = 0.03 and capillary number Ca = 10[superscript −8.6] to an end-of-drainage
brine saturation of 9%. We provide evidence of the applicability of previous two-dimensional
micromodel studies and ambient condition experiments in predicting flow regimes occurring during
scCO₂ injection.
Genre Article
Topic Supercritical CO₂
Identifier Herring, A. L., Andersson, L., Newell, D. L., Carey, J. W., & Wildenschild, D. (2014). Pore-scale observations of supercritical CO₂ drainage in Bentheimer sandstone by synchrotron x-ray imaging. International Journal of Greenhouse Gas Control, 25, 93-101. doi:10.1016/j.ijggc.2014.04.003

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