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Perturbed directional correlation in Ta-181

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Title Perturbed directional correlation in Ta-181
Names Sommerfeldt, Raymond Walter (creator)
Schecter, Larry (advisor)
Date Issued 1964-08-06 (iso8601)
Note Graduation date: 1965
Abstract The effect of a static quadrupole interaction on the 133-482 Kev
gamma-gamma angular correlation in Ta-181 has been studied by the
delayed coincidence method. Using a source of Hf-181 in polycrystalline
hafnium metal, the anisotropy was measured as a function of
time between the formation and decay of the 482 Key state with a
fast-slow coincidence spectrometer. The anisotropy as a function of
time revealed clearly the periodic fluctuations arising from the reorientation
of the nuclear spin due to coupling of the quadrupole
moment of the 482 Kev state with the electric field gradients of the
hafnium crystals. The interaction strength evaluated on the basis of
the theory of Abragam and Pound for axially-symmetric gradients
was 317 ± 8 Mc/sec. Evidence for the presence of a rhombic (non-axial symmetric) electric interaction was observed in the departure
of the results from the predictions of the axially-symmetric theory.
The results are, however, in agreement with the theory for rhombic interactions if the electric field gradient in the hafnium crystals used
is assumed to have an asymmetry parameter η = (V[subscript xx] - V[subscript yy])/V[subscript zz] = 0.3.
A similar study of the 133-345 Key gamma-ray cascade did not permit
a direct observation of the quadrupole coupling due to interference
from the 133-482 and 345-137 Key cascades; however, when the contributions
of the interfering cascades were removed from the composite
data, the results were consistent with those of the 133-482
experiment as well as with existing theory. An indirect determination
of the anisotropy of the 345-137 Key cascade gave the value 0.32 ± 0.02
in agreement with a previous measurement. In addition, the half-life
of the 482 Key excited state was remeasured to be 10.4 ± 0.2 nanoseconds
consistent with prior determinations.
Genre Thesis/Dissertation
Topic Nuclear physics
Identifier http://hdl.handle.net/1957/48372

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