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Examinations of ice formation processes in Florida cumuli using ice measurements of anvil ice crystal particle residues

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Title Examinations of ice formation processes in Florida cumuli using ice measurements of anvil ice crystal particle residues
Names Prenni, Anthony J. (creator)
DeMott, Paul J. (creator)
Twohy, Cynthia (creator)
Poellot, Michael R. (creator)
Kreidenweis, Sonia M. (creator)
Rogers, David C. (creator)
Brooks, Sarah D. (creator)
Richardson, Matthew S. (creator)
Heymsfield, Andrew J. (creator)
Date Issued 2007 (iso8601)
Note copyrighted by American Geophysical Union
Abstract A continuous flow diffusion chamber (CFDC) was used to measure ice formation by
cloud particle residuals during the Cirrus Regional Study of Tropical Anvils and Cirrus
Layers-Florida Area Cirrus Experiment. These measurements were directed toward
determining the relative contributions of homogeneous nucleation, heterogeneous
nucleation, and secondary ice formation processes to the concentrations of ice crystals in
anvil cirrus formed from convection. The CFDC sampled residual particles remaining
after evaporation of cloud particles initially collected by a counterflow virtual impactor.
This allowed, for the first time, determination of the ice nucleation ability of particles that
included the presumed nuclei for cloud-ice formation. The approach proved successful
for estimating concentrations of heterogeneous ice nuclei (IN) transported into anvil
clouds, but experimental issues limited measurements of homogeneous freezing and,
consequently, in determining the role of secondary ice formation. Results suggest
agreement within a factor of 2–3 between CFDC heterogeneous IN concentrations and
anvil ice crystal concentrations in the size range above ~30 μm. IN concentrations also
correlated with ice concentrations inferred from measurements by the FSSP (Forward
Scattering Spectrometer Probe). However, measured IN concentrations were nearly two
orders of magnitude lower than FSSP concentrations. This difference may have
resulted from homogeneous freezing, secondary ice formation, or other unidentified ice
formation processes that were not fully captured by the CFDC. The data suggest that
heterogeneous nucleation played a smaller role than homogeneous nucleation in
determining anvil ice crystal concentrations, except during periods of strong desert dust
ingestion by cumuli. Nevertheless, heterogeneous nucleation may provide the source for
larger ice crystals present in anvil regions.
Genre Article
Identifier Prenni, A. J., DeMott, P. J., Twohy, C. H., Poellot, M. R., Kreidenweis, S. M., Rogers, D. C., Brooks, S. D., Richardson, M. S. and Heymsfield, A. J., 2007, Examinations of ice formation processes in Florida cumuli using ice nuclei measurements of anvil ice crystal particle residues: J. Geophys. Res., v. 112, D10221

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